Complex-frequency pole analysis of resonance matching and heat redistribution in metal–polymer optical cavities
Applied Optics 65, 8734–8740
Complex-frequency resonance modes connect field localization and heat redistribution in optical cavities.
Abstract (original) · EN
Optical resonances in multilayer cavities arise from constructive interference of electromagnetic waves and govern field enhancement, energy localization, and photothermal energy conversion. Although resonance phenomena are commonly characterized through real-frequency spectral responses, their underlying modal structure remains insufficiently understood. Here, a complex-frequency framework is developed to investigate optical resonance modes in metal–polymer–metal (M–P–M) cavities. Analytical solutions of the frequency-domain Maxwell–Helmholtz equation are assembled through interfacial continuity conditions to construct a global fieldresponse function, whose poles define the intrinsic resonance modes of the cavity. The framework is applied to a Cr–PDMS–Cr cavity to investigate how complex-frequency resonance poles underlie resonance matching, field localization, and energy redistribution as functions of polymer-layer thickness, refractive index, and metal-layer thickness. Resonance matching to a 532 nm excitation wavelength is achieved through cavity-thickness tuning, and the corresponding complex-frequency resonance poles are systematically tracked as the structural and material parameters are varied. The pole-based predictions are validated by real-frequency electric-field calculations, confirming the correspondence between the resonance pole associated with the excitation wavelength and the resonance-matching condition. The results further show that refractive-index contrast and metal-layer attenuation govern resonance-pole migration and the resulting resonance characteristics of the cavity. Resonance matching produces strong electric-field localization within the polymer cavity while substantially reducing metallic heat generation through resonance-induced energy redistribution. These findings establish a consistent physical relationship between complex-frequency resonance poles and real-frequency optical and thermal responses, providing a unified modal framework for interpreting resonance matching, field localization, and resonance-mediated energy redistribution and a basis for the analysis and design of photothermal multilayer structures.
